Radioactivity and elemental analysis of carbonatite rocks from parts of Gwasi area, South Western Kenya
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Date
2009Author
Achola, Shem Opiyo
Type
ThesisLanguage
enMetadata
Show full item recordAbstract
Rocks and soils from a number of areas under lied by carbonatite rocks in Kenya have
been associated with high radioactivity. In this thesis, the analyzed results of the
background radiation measurements in the field, activity concentrations of primordial
radionuclides in the samples, approximated annual external effective dose rates and the
elemental concentrations of samples from Ruri hills have been presented. Ruri hills are
roughly between latitudes 0˚30’S and 1˚00’S, bounded on the east by longitude 34˚30’E
and on the west by the shores of Lake Victoria and the Winnam Gulf. Altitudes range
from about 1000m on the shores of Lake Victoria to above 1800m on top of the Ruri
hills. Gamma spectrometric analyses of twenty one samples from South and North Ruri
hills in Lambwe east location of Suba District, south western Kenya, have been carried
out using high-purity germanium (HPGe) gamma-ray detector. The samples comprise
rocks (mainly carbonatite) and soils. The activity concentrations ranged from 14.18 to
6559.99 Bqkg-1 with an average of 1396.85Bqkg-1 for thorium-232; from 2.73 to
499.24Bqkg-1 with an average of 178.69Bqkg-1 for uranium-238 equivalent; and from
56.67 to 1454.73Bqkg-1 with an average of 508.67Bqkg-1 for potassium-40. The
corresponding ranges of elemental concentrations, and the mean values in ppm are 25.151346.67,
280.04; 6.89-137.33, 27.91; and 438.00-3060.00, 1345.90; for thorium, uranium
and potassium respectively. Absorbed dose rates in air outdoors at approximately 1m
above the ground were measured using survey meters. The values are in the range of 700
to 6000.00nGyh-1, with an overall mean value of 2325.84nGyh-1. These values
correspond to individual annual effective dose rates ranging from 1.717 to 14.717mSvyr-1
with an overall mean of 5.705mSvyr-1, assuming a 40% (0.4) occupancy factor. Thus,
annual external effective dose rates at Ruri hills are much higher than the global average
of 0.46mSvyr-1 (i.e. approximately twelve times the global average).
Citation
Master of Science (Physics)Publisher
University of Nairobi School of Physical Sciences